Estimation of Unknown Source of Atmospheric Release
Monitoring airborne radioactivity involves determining the temporal profile and source characteristics of the release. While the location of the release is often known, the temporal profile and total quantity of the released substances are typically uncertain or only partialy known. This research focuses on reconstructing the temporal dynamics of a release using field measurements, such as concentration or deposition data. The methodology employs optimization techniques to compare observed measurements with numerical predictions from atmospheric dispersion models. Advanced Bayesian inference methods in machine learning, along with state-of-the-art deep neural networks, are utilized to enhance this process. Primary applications include the characterization of radionuclide releases from specific locations or estimation of complex spatial-temporal sources, such as emissions of ammonia or microplastics and microfibers.


Our Research
Our research is motivated by applications in radiation safety, particularly the estimation of unknown radionuclide emissions based on available measurements and the subsequent analysis of their dispersion using the inferred emissions. Specific examples include the estimation of releases during the Chernobyl accident, analyzing the iodine leak in Hungary in 2011, or the retrospective modeling of ruthenium releases from Siberia in 2017. Measurements and modeling of these events are often complicated by significant uncertainties and limitations in the available data, which are frequently incomplete and imprecise. We address these challenges by integrating all available information and uncertainties into inverse modeling frameworks based on Bayesian methods. This approach not only provides emission estimates but also quantifies their uncertainties, enabling an assessment of the reliability of the estimates derived from the available data.

An Additional Research Direction
An additional research direction focuses on complex spatiotemporal emissions, where releases may originate from any point within the computational domain. Examples include emissions of microplastics, ammonia, and wildfires around Chernobyl, which combine spatiotemporal sources with height-dependent releases and size-dependent particle distributions. These scenarios introduce new complexities in modeling and estimation, which can be addressed using Bayesian approaches or deep neural networks. Our results contribute to more accurate assessments of the environmental impacts of these emissions.
Related publications:
- TICHÝ Ondřej, ŠMÍDL Václav, HOFMAN Radek, ŠINDELÁŘOVÁ Kateřina, HÝŽA Miroslav, STOHL Andreas. Bayesian inverse modeling and source location of an unintended 131I release in Europe in the fall of 2011, Atmospheric Chemistry and Physics, 2017, 17.
- TICHÝ Ondřej, ŠMÍDL Václav, EVANGELIOU Nikolaos. Source term determination with elastic plume bias correction, Journal of Hazardous Materials 2022, 425.
- EVANGELIOU Nikolaos, TICHÝ Ondřej, ECKHARDT Sabine, GROOT ZWAAFTINK Christine, BRAHNEY Janice. Sources and fate of atmospheric microplastics revealed from inverse and dispersion modelling: From global emissions to deposition, Journal of Hazardous Materials, 2022, 432.
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